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It has been reported that MnSn2 exhibited unusual magnetic behaviors related to its crystal structure. However, little work has been done to investigate its behavioral responses to a high magnetic field (HMF), which is of potentially fundamental interest. Based on this, binary Sn­Mn alloy was solidified under different HMFs in this work. The results show that the primary MnSn2 crystals appear blockor bar-like shapes in both the longitudinal and transverse sections. In the longitudinal sections, however, the HMFs tend to align the bar-like crystals with the long axes perpendicular to the magnetic field. In the transverse sections, the HMFs have little influence on the alignments of the bar-like crystals but increase their amount. A crystallographic study indicates that ©110a is the easy magnetization axis of the MnSn2 crystals that orients preferentially parallel to the magnetic field. These results are attributed to the magnetic anisotropy of the MnSn2 crystals. [doi:10.2320/matertrans.M2019030]

Alignments and Orientations of MnSn<sub>2</sub> Phase during the Solidification Process of Sn–Mn Alloy under a High Magnetic Field