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We have operated a 4 Vclass bulktype, allsolidstate LiCoO2/Li battery at room temperature. The composition consisted of a Li4(BH4)3I complex hydride electrolyte for the electrolyte layer, and a 80Li2S 20P2S5 sulfide glass for an electrolyte in the positive electrode layer. The battery assembled exhibited a 92 mAh・g-1 initial discharge capacity at 298 K and 0.1 C. The discharge capacity for the 20th cycle remained as high as 83 mAh・g-1, corresponding to a capacity retention ratio of nearly 90. [doi:10.2320/jinstmet.JD201601]

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Development of 4V-Class Bulk-Type All-Solid-State Lithium Rechargeable Batteries by a Combined Use of Complex Hydride and Sulfide Electrolytes for Room Temperature Operation