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The volume of a quenched glassy alloy is a variable of cooling rates during the amorphization. Hence a change in the volume caused by the structural relaxation can be regarded as a degree of amorphousness. The density of Zr 50 Cu 40 Al 10 bulk glassy alloys (BGAs) increases linearly with the annealing temperature below the glass-transition temperature (T g ). With increasing the annealing temperature, the tensile strength and Vickers hardness show constant values, whereas the Young's moduli and Charpy impact values become larger and smaller, respectively. Especially, Charpy impact values of Zr-Cu-Al BGAs have a linear relationship with the relative value of excessive free volume, which correspond to the volume-change ratio caused by the full structural relaxation.

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Evolution of Mechanical Properties of Cast Zr&lt;SUB&gt;50&lt;/SUB&gt;Cu&lt;SUB&gt;40&lt;/SUB&gt;Al&lt;SUB&gt;10&lt;/SUB&gt; Glassy Alloys by Structural Relaxation