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We conducted X-ray and neutron diffraction experiments and magnetic susceptibility measurements for -MnFe alloys with a small amount of Cu or Pt, and for -MnCu and -MnZn alloys. -(Mn1 xFex)0:95Cu0:05 alloy with x 1⁄4 0:26 around 10K shows a face-centered orthorhombic structure with a 1⁄4 0:3681, b 1⁄4 0:3655 and c 1⁄4 0:3622 nm, and a non-collinear antiferromagnetic structure with a 1⁄4 0 and b= c 1⁄4 0:62. With increasing temperature, orthorhombic-tetragonal with c=a > 1 structural transition occurs at To (1⁄4 125K) and the tetragonal structure finally transforms to a cubic structure at Tt (1⁄4 352K), which is lower than the Neel temperature TN (1⁄4 440K). The (Mn1 xFex)0:95Pt0:05 alloy with x 1⁄4 0:13 at 10K also shows a similar structure with a 1⁄4 0:3745, b 1⁄4 0:3714 and c 1⁄4 0:3649 nm, which has a non-collinear antiferromagnetic structure with a 1⁄4 0, b 1⁄4 1:03 and c 1⁄4 1:94 b/(Mn or Fe) atom. The -Mn1 xCux alloy with x 0:26 and -Mn1 xZnx alloy with x 0:28 show a tetragonal structure with c=a < 1 at low temperature.

Crystal Distortion and Magnetic Structure of &gamma;-MnM (M = Fe, Cu, Zn) Alloys

Crystal Distortion and Magnetic Structure of γ-MnM (M = Fe, Cu, Zn) Alloys