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The electrochemical oxidation of carbon monoxide and the interfacial structure of the CO adlayer (CO a d s ) on platinum low index single crystals, Pt(111), Pt(100) and two reconstruction of Pt(110), were examined using the rotation disk electrode method in combination with the in situ surface X-ray diffraction scattering technique. The mechanism of CO oxidation is discussed on the basis of the findings that, depending on the potential, two energetic states of CO a d s exist on the platinum surfaces. Thus, at lower potentials, weakly bonded states (CO a d s , w ) and at higher potentials strongly bonded states (CO a d s , s ) are formed. The mechanism of the oxidation of hydrogen-carbon monoxide mixtures is also proposed.

journal of the serbian chemical society

Electrochemical oxidation of carbon monoxide: From platinum single crystals to low temperature fuel cells catalysts. Part I: Carbon monoxide oxidation onto low index platinum single crystals