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In this work, the random pore model was modified for a general concentration   dependency and also bulk flow effect, in order to predict the carbonation   reaction of calcium oxide with carbon dioxide. This reaction is one of the   main methods for carbon dioxide capture from industrial flue gases.   Different kinetic rate concentration functions were tested with the various   literature experimental data for finding the best reaction constants and   rate functions. Moreover, an exponential function for the diffusion of   carbon dioxide through the product layer was proposed from the whole   experimental conversion-time profiles

A modified random pore model for carbonation reaction of calcium oxide with carbon dioxide