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New spectroscopic technique which detects IR transition with high sensitivity is introduced asa tool to study laser reaction control by vibrational excitation. This spectroscopy, nonresonant ionization detectedIR spectroscopy is IR-UV double resonance spectroscopy which detects a vibrationally excited molecule by selective ionization due to UV laser. Vibrational transitions of jet-cooled phenol have been detected by Nonresonant Ionization Detected (NID)-IR spectroscopy from 3400 cm-1 to 14000 cm-1. The bandwidth of the OH overtone is found to decrease with increase in the vibrational quantum number. Relaxation of the vibrationally excited molecule and its application to reaction control are discussed.

Laser Detection of Vibrationally Highly Excited Molecules and Its Application to Reaction Control.