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Single crystal X-ray structure elucidation of the trinuclear module 4 and of the coordination polymer 5 reveals the presence of HS-LS-HS chains and all-HS infinite 1-D strands, respectively. As anticipated the presence of the bridging urea supports the supramolecular concatenation within an extended hydrogen-bonding network. Magnetic measurements reveal spin crossover behavior for four of the five complexes (1 – 4) that is strongly solvent dependent.

Iron(II) Spin Crossover Polymers of Planar N2O2 Schiff Base Templates and 4,4’-bis(pyridyl)urea Bridges