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This thesis is divided into two major parts. In the first part an experimental study of proton and deuteron transfer in H/sub 2//sup +/ + He and HD/sup +/ + He has been carried out as a function of kinetic and vibrational energy. The data gives evidence that at lower kinetic energies, the spectator stripping mechanism indeed plays an important role when H/sub 2//sup +/ or HD/sup +/ is vibrationally excited. The second half of this thesis examines the relative efficiencies between the excitation of C-C stretching vibration and collision energy on the promotion of the H atom transfer reaction of C/sub 2/H/sub 2//sup +/ + H/sub 2/ ..-->.. C/sub 2/H/sub 3//sup +/ + H.

Effect of collision energy and vibrational excitation on endothermic ion-molecule reactions