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Calculations have been made of the build-up of higher nuclides in samples of various heavy-element starting materials, at neutron fluxes ranging from 4 x 10/sup 13/ to 1 x 10/sup 16/ n/ cm/sup 2//sec, including the flux expected from the HFIR reactor at Oak Ridge (namely, 5 x 10/sup 15/ n/cm/sup 2// sec). Attempts have been made to estimate yields of the heavier fermium isotopes and of Md/sup 259/ by means of the nuclear properties predicted from systematics. The results indicate that it may be possible to detect Md/sup 259/ in the products of californium irradiated in HFIR, and that a further two-fold increase in flux would increase the yields of the heaviest nuclides considerably. (auth

CALCULATIONS OF YIELDS OF PRODUCTS IN HIGH-FLUX NEUTRON IRRADIATIONS OF HEAVY ELEMENT SAMPLES