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The understanding of crystal nucleation and growth has evolved over the past two decades from the conventional atom-by-atom model to a non-classical approach, involving particle aggregation and amorphous transformation pathways. Whereas aggregation of particles instead of individual atoms/ions/ molecules has been recognized as a common crystallization pathway at the Earth’s surface conditions, few cases are known for high-temperature (e.g., melt) mineralization, which is of great importance for understanding geological processes.

Evidence for a two-stage particle attachment mechanism for phyllosilicate crystallization in geological processes