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Modeling of ionic diffusion in natural crystals has been developed over the last three decades to calculate timescales of geological processes. As the number of studies and the size of data sets have expanded, improvements in the precision of the general technique are needed to resolve temporal patterns that would otherwise be masked by large uncertainties. This contribution examines fundamental aspects of timescale calculation uncertainty using Mg-Fe zonation in olivine crystals from a Piton de la Fournaise oceanite erupted in 2002 CE. First, we quantitatively consider the role of geometric uncertainty in data sets from the perspectives of sectioning angle, crystal shape, and crystal agglomeration. Second, we assess how crystal growth and changing boundary conditions during diffusion pose problems for simplistic, 1D, diffusion-only modeling.

american mineralogist

Reducing epistemic and model uncertainty in ionic inter-diffusion chronology: A 3D observation and dynamic modeling approach using olivine from Piton de la Fournaise, La Réunion