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The heat capacities, C 0  P , of synthetic rhodonite (MnSiO 3 ) and braunite (Mn 7 SiO 12 ) have been measured by adiabatic calorimetry from 6 to ~350 K. The heat capacity of braunite was also measured to ~900 K by differential scanning calorimetry. Braunite exhibits a λ-peak (paramagnetic to antiferromagnetic transition) in C 0  P  in the temperature region 93.4-94.2 K. Rhodonite did not show the expected peak in C 0  P  characteristic of the cooperative ordering of the Mn 2+  spins at temperatures above 6 K.

Heat capacities and thermodynamic properties of braunite (Mn 7 SiO 12 ) and rhodonite (MnSiO 3 )