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The cyclopalladated complex [Pd(C2,N-dmba)(μ-SCN)]2, where dmba = N,N-dimethylbenzylamine, was structurally characterized by single-crystal X-ray diffraction. This compound crystallizes in the monoclinic system, space group P21/n with a = 9.578(1)A, b = 12.323(2)A, c = 10.279(2)A, β = 117.03(1)°, V = 1080.7(3)A3, Z = 2. Each Pd(II) center displays a distorted square-planar coordination environment, formed by the C and N atoms from the dmba ligand, and one set of N and S atoms from the bridging SCN groups.

Molecular and Crystal Structure of Di(.MU.-N,S-thiocyanato)-bis[(N,N-dimethylbenzylamine-C2,N)palladium(II)]