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We report the red-emitting mechanoluminescence (ML) materials based on the piezoelectric semiconductors MZnOS:Mn2+ (M = Ca, Ba) synthesized by solid-state reaction. Both of the CaZnOS:Mn2+ and BaZnOS:Mn2+ show red light emission upon the compressive load, and the CaZnOS:Mn2+ emits a more intense red ML light at the same condition. We propose it should be considered to the polar non-centrosymmetric crystal structure of CaZnOS.

Mechanoluminescence properties of red-emitting piezoelectric semiconductor MZnOS:Mn<sup>2+</sup> (M = Ca, Ba) with layered structure