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The development of electric vehicles and portable electronic devices demand lighter and thinner batteries with improved specific charge and rate capabilities. In this work, we prepared LiNi0.3Co0.3Mn0.3O2 (NCM) using a co-precipitation route. Li1.3Al0.3Ti1.7(PO4)3(LATP) was synthesized using a solid state reaction method. LiNi0.3Co0.3Mn0.3O2-Li1.3Al0.3Ti1.7(PO4)3 (NCM-LATP) composites, with spherical agglomerates of NCM particles being homogenously dispersed in microsized LATP matrix, had been prepared by dielectric barrier discharge plasma assisted milling (DBDPmilling) for the first time. We analyzed surface morphologies and structures of the LATP, NCM and NCM-LATP samples by using scanning electron microscopy (SEM) and X-ray diffraction (XRD). We analyze performances of model NCM-LATP materials. The results show that the NCM-LATP composites exhibits excellent cycles tability to reach 127.4, 118.7 and 109.5 mAh g -1 at 0.2, 0.5 and 1C (at room temperature), respectively. The NCM-LATP composites cathode and NCM cathode had a discharge capacity of 155.9 and 136.2 mAh g -1 at the first cycle, and the corresponding coulombic efficiencies are 92.96% and 74.75%, at 0.05 C. Charge-discharge curves, Cyclic voltammetry and AC impedance response indicated that both NCM and LATP phases in the composite cathode were involved during the oxidation-reduction reactions and the electron transport resistance in the pure NCM cathode was much higher than that in the NCM-LATP composites cathode.

Electrochemical Performance of LiNi0.3Co0.3Mn0.3O2-Li1.3Al0.3Ti1.7(PO4)3 Composites Prepared by Dielectric Barrier Discharge Plasma Assisted Milling