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Li6PS5Cl-coated Li4Ti5O12 materials was fabricated by a simple liquid-phase treatment method. Charge-discharge tests show that Li6PS5Cl-coated Li4Ti5O12 (LTO@LPSCl)/Li6PS5Cl/Li all-solid-state lithium batteries exhibit high reversible capacity (~158 mA h·g -1 ) after 250 cycles under 0.05 C and excellent rate capacity (~50 mA h·g -1 ) under 1 C at 80 °C .A combination of scanning electron microscopy (SEM), energy dispersive X-ray analysis (EDX) mapping, and electrochemical impedance spectra (EIS) reveals that good wettability of liquid with Li4Ti5O12 materials and Li6PS5Cl is responsible for Li6PS5Cl nanoparticle coated on the surface of Li4Ti5O12 materials homogenously, which build the stable interface between active materials and solid state electrolyte, reduce the interface resistance effectively, and result in excellent electrochemical performances.

Fabrication and Electrochemical Properties of Li4Ti5O12@Li6PS5Cl for All-solid-state Lithium Batteries using Simple Mechanical Method