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ELECTROCHEMICALLY -FABRICATED METAL NANOSTRUCTURES FOR SENSING, RESISTIVE SWITCmNG, RAMAN ENHANCEMENT, AND MAKING CONTACT TO MOLECULAR JUNCTIONS RADmKA DASARI (AUGUST 03 2011) The research in this dissertation describes a simple electrochemical approach for fabricating nanoscale (metal/metal) or molecular (metal/polymer or self assembled monolayer (SAM)/metal) junctions. The fabrication involves metal deposition on one set of electrodes (El), where the metal grows and becomes connected to a second set of electrodes (E2) of an Au interdigitated array of electrodes with a 5 11m separation. The fabrication of molecular junctions involves deposition of a thin polymer or self assembled monolayer film on one set of electrodes (E2) prior to metal deposition on the other set of electrodes (El). The method is simple, low cost, highly parallel, and applicable to a wide variety of molecules and thin films with interesting electronic properties. Different metal/metal and metal/molecule or polymer/metal junctions such as Ellnano PdlE2, Ellnano PdlpolyphenollE2, ElIAg nanowire(NW)1E2, ElIAgNW/polyphenollE2 and ElIAgNW/SAMlE2 junctions were fabricated using this

Electrochemically-fabricated metal nanostructures for sensing, resistive switching, Raman enhancement, and making contact to molecular junctions.