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Catalytic performance of nickel-loaded zeolite-based supports for CO2 reforming of methane was investigated. Among the three zeolites (H-Y, H-mordenite, and Na-mordenite), H-mordenite was the best support for the reaction, probably due to its thermal stability. The initial activity of Ni/H-mordenite (Ni/HM) was higher than that of conventional Ni/alumina catalyst (Ni/Al2O3), whereas deactivation of the former was slightly faster. A physical mixture of alumina and zeolite was a more effective support than zeolite. The resulting Ni/H-mordenite-alumina catalyst (Ni/HM-Al2O3) showed the highest performance among the catalysts tested. Under the conditions of atmospheric pressure of CO2/CH4/He stream (20/20/40ml/min)at 750°C, the initial CO2 conversion was 95% and this value was maintained for more than 20h. The catalytic performance of Ni/HM-Al2O3 was higher than that of Ni/Al2O3.

Reforming of Methane with Carbon Dioxide over Nickel-loaded Zeolite Catalysts.