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Accurate potential energy curves, transition moments, spectroscopic constants, radiative transition probabilities, and lifetimes for the states X2S+ and A2P of BeF, MgF and CaF are reported using high level calculations. Diagonal transitions dominate for the A2P ® X2S+ system. Radiative lifetimes for n' = 0 are predicted to be 6.81 ns, 7.16 ns and 19.48 ns, respectively for BeF, MgF and CaF. The result calculated for the CaF molecule are in excellent agreement with the experimental result equal to 21.9±4.0 ns.

Radiative transition probabilities and lifetimes for the band systems A²pi - X²sigma+ of the isovalent molecules BeF, MgF and CaF