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i DEDICATION  iv ACKNOWLEDGEMENTSv LIST OF TABLES  viii LIST OF FIGURES  ix CHAPTER 1: Introduction 1 1.1 Background 1 1.2 Purpose and Relevance of this Research 7 1.3 Reader’s Guide to the Thesis 8 CHAPTER 2: Geochemical status of a remedial cap on creosote-contaminated sediments at the McCormick and Baxter Superfund Site and its potential link to natural attenuation ..10 2.1 Executive Summary 10 2.2 Methods11 2.3 Results and Discussion 15 2.4 Conclusions23 CHAPTER 3: Detection of anaerobic metabolites of naphthalene degradation at a creosotecontaminated Superfund site and in situ transformation of deuterated naphthalene to a naphthoic acid analogue 28 3.

Anaerobic Degradation of Polycyclic Aromatic Hydrocarbons at a Creosote-Contaminated Superfund Site and the Significance of Increased Methane Production in an Organophilic Clay Sediment Cap