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We report our determination of molecular constants for the 21Π state of NaLi from set of 732 spectral lines. Using the linear least-squares fitting method, an optimum set of molecular constants, which corresponds to dimensionless root mean of squares of deviation σ = 0.62 within 0.1 cm-1 experimental uncertainty, have been derived.

Molecular Constants of the 2\(^1\Pi\) State of \(\text{NaLi}\) Molecule