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Besides graphite and diamond, the solid allotropes of carbon in sp2 and sp3hybridization, the possible existence of a third allotrope based on thesp-carbon linear chain, the Carbyne, has stimulated researchers for a longtime. The advent of fullerenes, nanotubes and graphene has opened newopportunities and nurtured the interest in novel carbon allotropes includinglinear structures. The efforts made in this direction produced a number ofinteresting sp-hybridized carbon molecules and nanostructures in the form ofcarbon-atom wires. We here discuss some of the new perspectives opened by therecent advancements in the research on sp-carbon systems.

Carbyne: from the elusive allotrope to stable carbon atom wires