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Basic principles of growing the thick (35–60 μm) single-crystalline La-substituted yttriumiron garnet (Y3−xLaxFe5O12, La :YIG) films with reproducible parameters have been formulated. La :YIG films are grown on gallium-gadolinium garnet (Gd3Ga5O12) substrates from a supercooled melt-solution (MS) consisting of Y2O3, La2O3, and Fe2O3 oxides and the PbO– B2O3 solvent. In order to minimize the implantation of Pb ions into the films, which degrades the film quality, the epitaxy has to be performed at high temperatures and a low MS supercooling. It is found that, in order to maintain a constant growth rate of La :YIG films with reproducible parameters, a large MS mass (10–16 kg) has to be used, and the MS temperature has to be permanently lowered at a rate of 0.042 K/min.

Growing of Thick Single-Crystalline La-Substituted Yttrium-Iron Garnet Films with Reproducible Parameters