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This paper gives an overview of the theory and some selected applications of the Multi-Configuration Time-Dependent Hartree-Fock(MCTDHF) method. This method can be seen as an explicitly time-dependent version of the Complete Active Space Self-ConsistentField (CASSCF) method of standard quantum chemistry. Strengths and shortcomings are discussed, and some comparisons with othermethods of correlated electron dynamics are given.

Ab initio Electron Dynamics with the Multi-Configuration Time-Dependent Hartree-Fock Method