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In this chapter, the Solid Electrolyte Interphase (SEI) concept is introduced and the different requirements on the electrolyteand on the SEI formation process in the presence of various anode materials (metallic lithium, graphitic carbons, and lithiumstorage metals/alloys), in particular, similarities and differences, are highlighted. The difficulties to understand and analyzethe SEI characteristics and composition are discussed by examples.

The Solid Electrolyte Interphase – The Most Important and the Least Understood Solid Electrolyte in Rechargeable Li Batteries