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Partially restricted coupled cluster calculations involving connected triple substitutions have been carried out for linear SiC 3  and SiC 5  in their  3 Σ -  electronic states. Both species are of substantial interest to interstellar cloud chemistry. Accurate equilibrium structures are established and the equilibrium dipole moments of linear SiC 3  and SiC 5  are predicted to be -4.49 D and -6.20 D, with the positive ends of the dipoles at the silicon sites. Various spectroscopic constants are predicted for different isotopomers of SiC 3 .

Linear Triplet SiC 3 and SiC 5 : Results of Coupled Cluster Calculations