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The linear electro-optic tensor [ r ijk  σ  ] (unclamped) and the tensor of linear electrostriction [ d ijk  ] were determined for the isotypic title compounds (point group [unk]2 m ) at room temperature and  λ  = 633 nm. Small electro-optic coefficients (one seventh to one tenth of those of KDP), small electrostrictive components (like  d  111  of  α -quartz) and high electro-optic anisotropy ( r  123 / r  231  ≫ 1) are the main features of these complex thiosulphates.

zeitschrift für kristallographie - crystalline materials

Electro-optic and electrostrictive properties of the complex thiosulphates (NH 4 ) 9 [Cu(S 2 O 3 ) 4 ]Br 2 , (NH 4 ) 9 [Cu(S 2 O 3 ) 4 ]I 2 , and (NH 4 ) 9 [Ag(S 2 O 3 ) 4 ]Br 2