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Single crystals of guanidinium tetrafluoroborate of optical quality and dimensions up to 60 × 60 × 30 mm have been grown from aqueous solutions. They possess a distinct polar morphology of point symmetry group 3 m  and strong pyroelectric, piezoelectric, electrooptic and nonlinear optic effects similar to those observed in hexagonal guanidinium iodide.

Pyroelectric, dielectric, piezoelectric, and elastic properties of trigonal guanidinium tetrafluoroborate, C(NH 2 ) 3 BF 4