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The cation-exchange behavior of  261 Rf ( T  1/2 = 78 s) produced in the  248 Cm( 18 O, 5 n ) reaction was studied on a “one-atom-at-a-time” scale in 0.15–0.69 M H 2 SO 4 /HNO 3  mixed solutions ([H + ]=1.0 M) using an automated ion-exchange separation apparatus coupled with the detection system for alpha-spectroscopy (AIDA). It was found that adsorption probabilities ( decrease with an increase of [HSO 4  − ], showing a successive formation of Rf sulfate complexes. Rf exhibits a weaker complex formation tendency compared to the lighter homologues Zr and Hf. This is in good agreement with theoretical predictions including relativistic effects.

Sulfate complexation of element 104, Rf, in H 2 SO 4 /HNO 3 mixed solution