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The interactions of pentavalent Np and Pu with nitrate ligands has been investigated in perchlorate/nitrate media by capillary electrophoresis-inductively coupled plasma mass spectrometry (CE-ICP-MS). The binding constant for the complex PuO 2 NO 3 , log 10 β PuO 2 NO 3  °=0.14±0.14, is established for the first time while a new value for NpO 2 NO 3 , log 10 β NpO 2 NO 3  °=0.13± 0.14, is proposed. The usual analogy applied between Np(V) and Pu(V) interactions seems to be valid for nitrates.

Determination of the stability constants of nitrate complexes of Np(V) and Pu(V) using CE-ICP-MS