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The radionuclide   64 Cu ( T  1/2 =12.7 h) is an important non-standard positron emitter, suitable for combining PET imaging and targeted therapy. Its production in no-carrier-added form is done   via   charged particle induced reactions, and considerable amount of cross section data are available in the literature. We evaluated seven reactions, namely  64 Ni( p ,  n )  64 Cu,   64 Ni( d , 2 n )  64 Cu,  68 Zn( p , α n )  64 Cu,   66 Zn( p , 2 n )  64 Cu,  64 Zn( d , 2 p )  64 Cu,   66 Zn( p , α)  64 Cu and  nat Zn( d ,  x )  64 Cu. Data analysis was generally limited up to about 25 MeV and the consistency check of experimental data was carried out using the nuclear model codes STAPRE, EMPIRE and TALYS. In a few cases experimental data were available up to 100 MeV; the consistency check in the high energy region was done only using the code TALYS. A statistical procedure (supported by nuclear model calculations) was then used to fit the data. The derived recommended sets of data, together with 95% confidence limits, are reported. The integral yields calculated from those data are also given. A critical comparison of the various production routes of   64 Cu is presented. The   64 Ni( p ,  n )  64 Cu reaction, utilizing a highly enriched target, is the method of choice.

radiochimica acta

Charged particle induced reaction cross section data for production of the emerging medically important positron emitter  64 Cu: A comprehensive evaluation