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In order to enhance the understanding of redox reactions of plutonium ions in molten NaCl-CsCl eutectic, absorption spectrophotometry was performed for Pu 3+ , Pu 4+ , and PuO 2  2+  in molten NaCl-CsCl at 923 K by controlling the flow-rate ratio of Cl 2  and Ar or O 2  in the ventilating mixture gas. Based upon the relations of the measured rest potentials to the concentration ratios of [Pu 4+ ]/[Pu 3+ ] and [PuO 2  2+ ]/[Pu 4+ ], the redox potentials of Pu 4+ /Pu 3+  and PuO 2  2+ /Pu 4+  couples in molten NaCl-CsCl eutectic at 923 K were estimated.

Redox equilibria of Pu 4+ /Pu 3+ and PuO 2 2+ /Pu 4+ couples in molten NaCl-CsCl eutectic as measured by absorption spectrophotometry