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Obtaining reliable thermodynamic data for Pu(V) is difficult because of its redox and/or disproportionation reactions in most aqueous systems. The known stability of Pu(V) in PuO 2 (am) suspensions in slightly acidic to near neutral conditions was used to study the solubility of PuO 2 (am) in 0.4 and 4.0 M NaCl or NaClO 4  solutions ranging in p c  H +   values from 4 to 9 as a function of time. The close agreement between the observed solubility and the predicted solubility using Pitzer ion-interaction parameters of Np(V) with Cl -  or ClO 4  -  for Pu(V) indicates that Pu(V), as expected, behaves in an analogous fashion to Np(V) and confirms the value of using Np(V) data to model Pu(V) behavior.

Thermodynamics of the PuO 2 + -Na + -OH - -Cl - -ClO 4 - -H 2 O system: use of NpO 2 + Pitzer parameters for PuO 2 +