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The ambient atmosphere is found to influence the thermal annealing behaviour of neutron-irradiated bissalicylaldehyde- triethylenetetramine Co(III) chloride, hydrate. The electron-donors, acetone and ethyl alcohol vapours, accelerate the annealing process, while electron-acceptors like oxygen and nitric oxide gas retard it. Evidently, a donor-acceptor electron transfer takes place between the crystallite and the adsorbed molecules of the ambient gas or vapour. It supports an annealing mechanism invoking participation of free electrons.

radiochimica acta

Influence of Electron-Accepting and Donating Ambient Atmospheres on the Thermal Annealing of Recoil Damage in Cobalt Chelates-bis-Salicylaldehyde-Triethylenetetramine Co(ni) Chloride, Hydrate