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Chemical reactions of hot atomic iodine formed by recoil from a photoneutron emission process, (γ, n) have been studied. The yield of the hot substitution,  126 I + CH 3 I → CH 3  126 I + I was determined. The probability of this process, compared to analogous reactions of hot hydrogen atoms, was found to be low. A possible reason for what appears to be a generally low efficiency of gas phase hot halogen atom substitution reactions is discussed.

The Hot Iodine Substitution Reaction in Gaseous Methyl Iodide