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Dipole oscillator strength distributions are constructed for CF 4 , CClF 3 , CCl 2 F 2 , CCl 3 F, CHF 3 , CH 3 F, CH 3 Cl, CH 3 Br, CH 3 I, C 2 F 6 , and CCl 3 CF 3  from experimental and theoretical photoabsorption cross-sections combined with constraints provided by the Kuhn–Reiche–Thomas sum rule, the high-energy behavior of the dipole-oscillator-strength density, and either molar refractivity data or static dipole polarizabilities depending upon the availability of refractivities. The distributions are used to predict dipole sum rules  S ( k ), mean excitation energies  I ( k ), and van der Waals  C  6  coefficients. Pseudospectral representations of the DOSDs are reported.

zeitschrift für physikalische chemie

Constrained Dipole Oscillator Strength Distributions for CF 4 , CClF 3 , CCl 2 F 2 , CCl 3 F, CHF 3 , CH 3 F, CH 3 Cl, CH 3 Br, CH 3 I, C 2 F 6 , and CCl 3 CF 3