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A new Co(II) complex, [Co(pta)(H 2 O) 2 ]  n   ( 1 ), with the 2-(4-pyridyl)-terephthalate ligand (pta 2− ) has been synthesized and structurally and magnetically characterized. Single crystal X-ray analysis indicates that the unique Co(II) ion in the asymmetric unit of  1  displays stretched octahedral geometry. Compound  1  presents a bimetallic layer structure which is further expanded to a 3D supramolecular network through hydrogen bonding interactions. Magnetic measurements have revealed the temperature-dependent existence of antiferromagnetic and ferromagnetic interactions in compound  1 .

A new Co(II) coordination polymer with the 2-(4-pyridyl)-terephthalate ligand: synthesis, crystal structure and magnetic properties