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Dimeric anilidolithium (ArHNLi·Et 2 O) 2  (Ar=2,6-  i  Pr 2 C 6 H 3 ) reacted with zirconium tetrachloride in THF to give the heterometallic zirconium–lithium complex [(Et 2 O) 2 Li(μ-Cl) 2 (ArHN)(ArN=)Zr(μ-Cl)] 2  ( C1 ) and with titanium tetrachloride in toluene to give the titanium complex [(ArN=)TiCl 2 ·(Et 2 O) 2 ] ( C2 ) each in good isolated yields. Their molecular structures in the solid state were confirmed by X-ray diffraction analysis. Upon activation with methylaluminoxane, both arylimido zirconium and titanium complexes exhibited good catalytic activities toward ethylene polymerization.

Arylimido zirconium and titanium complexes: characteristic structures and application in ethylene polymerization