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A new tetradentate Schiff base-like ligand H2L (1) ((E,E)-dimethyl-2,2´-[1,2-phenylenebis(aminomethylidyne)] bis[3-oxobutanoate]) was synthesised and structurally characterised. Its reaction with iron(II) acetate leads to the formation of the octahedral N 2 O 4 -coordinated complex [FeL(MeOH) 2 ] (2). The complex is a pure high-spin (HS) compound as is evident from magnetic measurements and X-ray crystallography.

A Promising New Schiff Base-like Ligand for the Synthesis of Octahedral Iron(II) Spin Crossover Complexes