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Reactions of silver(I) salts with 4-amino-4H-1,2,4-triazole (4-NH 2 -tz) in a 1 : 1 molar ratio yield four new silver adducts, namely [Ag(4-NH 2 -tz)](CF 3 SO 3 ) (1), [Ag(4-NH 2 -tz) 1.75 ](ClO 4 ) (2), [Ag(4- NH 2 -tz) 1.75 ](BF 4 ) (3) and [Ag(4-NH 2 -tz) 1.75 ](NO 3 ) (4). X-Ray analysis shows that 1 exhibits a 3D cationic [Ag(4-NH 2 -tz)] +  metal-organic framework of srs topology; 2, 3 and 4 are isostructural and display an infinite chain structure containing an Ag 4 tz 6  cluster.

Synthesis and Structures of Silver(I) Adducts with 4-Amino-4H-1,2,4-triazole