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The new binary alkaline earth rich indides Ca 2 In (orthorhombic, space group Pnma, a =727.5(2), b = 537.1(2), c = 999.0(3) pm, Z = 4, R1 = 0.0252, Co 2 Si structure type) and Sr 28 In 11  (orthorhombic, space group Imm2, a=582.6(3), b=6687.8(9), c=823.5(6) pm, Z =2, R1=0.0571, Ca 28 Ga 11  structure type) have been synthesized from stoichiometric melts of the elements. Both crystal structures exhibit isolated In atoms coordinated by seven to ten alkaline earth atoms. In the crystal structure of Sr 5 In 3  (tetragonal, space group I4/mcm, a = 874.4(3), c = 1642.9(8) pm, Z = 4, R1 = 0.0347, Cr 5 B 3  structure type) isolated In atoms coexist with In 2  dumbbells exhibiting short In-In contacts (284.4 pm). The electronic structures of the less elaborate compounds Ca 2 In and Sr 5 In 3  are discussed in comparison with those of the closely related, nominally electron precise Zintl compounds Ca 2 Sn and Sr 5 Sn 3 .

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Neue Erdalkalimetall-reiche binäre Indide: Ca 2 In, Sr 28 In 11  und Sr 5 In 3  / New Alkaline Earth Rich Binary Indides:  Ca 2 In, Sr 28 In 11  und Sr 5 In 3