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The preparation, crystal structures, optical absorption spectra, and photoluminescence spectra of the title compounds are reported. The compounds were prepared in single crystal form. [C 6 H 5 CH 2 NH 3 ] 2 PbI 4  consists of anionic perovskite sheets of corner-sharing Pbl 6  octahedra, which alternate with the C 6 H 5 CH 2 NH 3  +  sheets. [ C 6 H 5 CH 2 CH 2 SC(NH 2 ) 2 ] 3  PbI 5  consists of zig-zag chains of anionic corner sharing PbI 6  octahedra separated by C 6 H 5 CH 2 CH 2 SC(NH 2 ) 2  cations. [C 10 H 7 CH 2 NH 3 ]Pbl 3  consists of twin chains of edge-sharing PbI 6  octahedra separated by C 10 H 7 CH 2 NH 3  cations. The compounds are thus low-dimensional systems. The excitonic spectra were observed in all cases, even at room temperature, and the possibility of organicinorganic excitonic interactions is discussed.

zeitschrift für naturforschung b

Preparation and Characterization of [C 6 H 5 CH 2  NH 3 ] 2 PbI 4 , [C 6 H 5 CH 2 CH 2 SC(NH 2 ) 2 ] 3  PbI 5  and [C 10 H 7 CH 2 NH 3 ]PbI 3  Organic-Inorganic Hybrid Compounds