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The preparation and characterization of three homologous actinidocenes of the composition An[η 8 -C 8 H 5 (SiMe 3 ) 3 -1,3,5] 2  (An = Th (1), U (2), Np (3)) is reported. Due to the presence of six trimethylsilyl groups these sandwich complexes are quite volatile and soluble in non-polar organic solvents.

Organoactinide Chemistry: Polysilylated Actinidocenes of Thorium, Uranium, and Neptunium