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From the results of magnetic susceptibility and magnetization measurements of the triple chains ACrF 4  (A = K, Rb, Cs), the characteristics of one-dimensional antiferromagnetic chains are found. The exchange parameters J/k are —6.2 K and —12.2 K for KCrF 4  and CsCrF 4 , respectively. Measurements on single crystals of RbCrF 4  reveal the exchange and the anisotropy parameters to be J/k = —10.5 K and D/k = 0.4 K. The Mössbauer spectra of 2%  57 Fe doped CsCrF 4  show marked relaxation. One third of the magnetic chains are frustrated and remain uncorrelated with other magnetic chains.

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Magnetische Untersuchungen an ACrF 4 -Verbindungen mit A = K, Rb, Cs  57 Fe-Mößbauer-Spektren von CsCrF 4  / Magnetic Studies of the Compounds ACrF 4  (A = K, Rb, Cs) A Mössbauer Study of  57 Fe-Doped CsCrF 4