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The hydrogen isocyanide complexes [M (CO) 5 CNH] (M = Cr, Mo, W) have been treated with the aziridines R [xxx] H 2  (R = H, R’ = H, Me, Et; R = Me, R’ = H) to give imidazolidin-2-ylidene complexes. The same type of ligand forms on addition of aziridine to the electrophilic isocyanide group in [FpCNPh] +  in the presence of Br − , IR,  1 H NMR,  13 C NMR and mass spectra of the new compounds are reported.

zeitschrift für naturforschung b

Chemie der Isoblausäure, II Reaktionen von [M(CO) 5 CNH] (M = Cr, Mo, W) mit Aziridinen: Zyklische Diaminocarbenkomplexe / Chemistry of Hydrogen Isocyanide, II Reactions of [M(CO) 5 CNH] (M = Cr, Mo, W) with Aziridines: Cyclic Diaminocarbene Complexes