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UV photoelectron spectra of the title compounds are reported. Assignments are made with the help of He(I)/He(II) intensity differences, shift effects upon substitution and comparison with related molecules. Previously drawn conclusions about the electronic structure of similar com­plexes also hold for the compounds. It is indicated that the ionization energy for the symmetric metal-metal bond strongly depends on the overlap between transition and post-transition metals.

The He(I) and He(II) Photoelectron Spectra of Tm 2 Zn (Tm = (C 5 H 5 )Fe(CO) 2 , (C 5 H 5 )M(CO) 3 ; M = Cr, Mo, W)