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⊿G for the reaction R ·+  + R ·-  → 2 R + ⊿G was calculated according to ⊿G = -(IP-EA) = -⊿ E 1  for the reaction in gas phase under ideal conditions. The result was compared with ⊿H in solution measured calorimetrically and the entropy term measured voltammetrically according to ⊿G = ⊿H - T⊿S. Both values for ⊿G agreed satisfactorily. From this it was derived that the solvation energies of R ·+  and R ·-  compensate mutually. The Coulomb energies have little influence on ⊿G only

Energiebilanz einer Reaktion zwischen Radikal-Kation und Radikal-Anion / Energy Turnover of a Reaction between Radical Cation and Radical Anion