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The crystal structure of a phosphorusnitrogen compound with two-coordinate cationic phosphorus was determined from single crystal X-ray data. The structure of the molecule shows two very short P–N distances (161.4 pm) indicating 3p π (P)— 2pπ(N) interaction between the phosphorus and the lone pairs of the nitrogen atoms. The N–P–N angle was found to be 97.4°.

zeitschrift für naturforschung b

Notizen: Kristallstruktur einer Phosphor-Stickstoff-Verbindung mit zweifach koordiniertem, kationisch stabilisierten Phosphor / Crystal Structure of a Phosphorus-Nitrogen Compound with Two-Coordinate Cationic Phosphorus