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Phosphorus-31 and carbon-13 chemical shifts as well as  31 P -  13 C and  31 P -  29 Si coupling constants have been obtained from a series of ten N -trim ethylsilyl-triorganophosphine imines. The influence of alkyl substituents on the phosphorus-31 chemical shifts in these and a variety of other com pounds is explained by a mechanism of intram olecular coordination of the β-CH 3  group to phosphorus using d-orbitals.

zeitschrift für naturforschung b

31 P- und  13 C-Kernresonanzuntersuchungen an N-Trimethylsilyl-triorganophosphiniminen / Phosphorus-31 and Carbon-13 Nuclear Magnetic Resonance Investigations of N-Trimethylsilyl Triorganophosphine Imines